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1 Comparison of SPR and LSPR Sensors FeatureCharacteristic Label-free detection Distance dependence Refractive index sensitivity Modes Temperature control Chemical identification Field portability Commercially available Cost Spatial resolution Nonspecific binding Real-time detection Multiplexed capabilities Small molecule sensitivity Microfluidics compatibility SPR Yes [25,27,35,40] 1000 nm [23] 2 106 nmRIU [3,23,24,26] Angle shift[22] Wavelength shift Imaging Yes SPR-Raman No Yes 150K300K 10 mm 10 mm [22,44] Minimal (determined by surface chemistry and rinsing) [3,22,3941] Timescale 14 101103 s, planar diffusion [24,25,39,42,43] Yes [45,46] Good [24] Yes LSPR 30 nm (size tunable) [60,61] 2 102 nmRIU [57,60] Extinction [56] Scattering [58,62] Imaging [58,62] No LSPR-SERS Yes No 5K (multiple particles); 50K (single nanoparticle) 1 nanoparticle [58,62,63] Minimal (determined by surface the best intraday Forex strategies on and rinsing) [56] Timescale 14 101103 s, radial diffusion [58] Yes (possible) Better [60] Possible lower refractive index sensitivity, color, and biochemistry.

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